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On Friday, Miller died of an apparent drug overdose in his home.
In a profile article published the day before his death by Vulture, Miller said, "I used to rap super openly about really dark sh- because that's what I was experiencing at the time".
Grande and Miller started seeing each other in 2016, three years after they first worked together on Grande's hit debut single "My Way".
The sudden news of Mac Miller's death continues to affect fans and artists who loved the late Pittsburg star, who once bragged, "I'm still playing it out the same speakers/I did it all without a Drake feature", on his 2014 track "Here We Go".
A statement from his family later read: 'Malcolm McCormick, known and adored by fans as Mac Miller, has tragically passed away at the age of 26.
Grande and Miller dated for around two years before breaking up earlier this year.
The Los Angeles Police Department told CNN that officers responded to a call for a death investigation at the 11600 block of Valleycrest Road just before noon local time Friday (Sept. 7). "At this time, an autopsy is pending and a cause of death has not been determined".
"I have cared for him and tried to support his sobriety and prayed for his balance for years (and always will of course) but shaming/ blaming a woman for a man's inability to keep his s*** together is a very major problem".
That he was battling addiction and struggling with depression was brought to light in his final interview with Vulture that was published Thursday.
"A lot of times in my life I've put this pressure to hold myself to the standard of whatever I thought I was supposed to be, or how I was supposed to be perceived", he told the NY magazine's Vulture website.
Mac Miller had previously released 3 new songs about Ariana Grande! Among them: Wiz Khalifa, G-Eazy and Chance the Rapper.
'Rest in your peace Mac Miller, ' Solange wrote.